From 1718d434efae26de02754c6622c43f4dc9e624b9 Mon Sep 17 00:00:00 2001
From: jranke <jranke@edb9625f-4e0d-4859-8d74-9fd3b1da38cb>
Date: Thu, 15 Mar 2012 15:54:14 +0000
Subject: Update kinfit and mkin to the latest version published on BerliOS.

git-svn-id: svn+ssh://svn.r-forge.r-project.org/svnroot/kinfit/pkg/mkin@17 edb9625f-4e0d-4859-8d74-9fd3b1da38cb
---
 DESCRIPTION                    |    25 +-
 R/DFOP.solution.R              |     5 +
 R/FOMC.solution.R              |     4 +
 R/HS.solution.R                |     6 +
 R/SFO.solution.R               |     4 +
 R/SFORB.solution.R             |     9 +
 R/mkin_long_to_wide.R          |    23 +-
 R/mkin_wide_to_long.R          |    20 +
 R/mkinerrmin.R                 |    20 +
 R/mkinfit.R                    |   398 +-
 R/mkinmod.R                    |   154 +-
 R/mkinplot.R                   |    83 +-
 R/mkinresplot.R                |    54 +
 R/mkinstart.R                  |    23 +
 inst/GUI/.RData                |   Bin 0 -> 17960 bytes
 inst/GUI/.Rhistory             |     3 +
 inst/GUI/gdf-test.R            |    12 +
 inst/GUI/simple-Gtk.R          |    33 +
 inst/GUI/simple.R              |    68 +
 inst/GUI/test.R                |    17 +
 inst/doc/Rplots.pdf            | 23902 +++++++++++++++++++++++++++++++++++++++
 inst/doc/mkin.Rnw              |    25 +-
 inst/doc/mkin.pdf              |   Bin 176018 -> 178902 bytes
 inst/doc/references.bib        |     7 +
 inst/unitTests/runit.mkinfit.R |    28 +-
 inst/unitTests/runit.mkinmod.R |    61 +-
 man/DFOP.solution.Rd           |    36 +
 man/FOCUS_2006_datasets.Rd     |     2 +-
 man/FOMC.solution.Rd           |    49 +
 man/HS.solution.Rd             |    34 +
 man/SFO.solution.Rd            |    29 +
 man/SFORB.solution.Rd          |    36 +
 man/mkin_long_to_wide.Rd       |     7 +-
 man/mkinerrmin.Rd              |     1 -
 man/mkinfit.Rd                 |    31 +-
 man/mkinmod.Rd                 |    18 +-
 man/mkinplot.Rd                |     6 +-
 man/mkinresplot.Rd             |    64 +
 man/mkinstart.Rd               |    38 +
 man/summary.mkinfit.Rd         |    16 +-
 tests/doRUnit.R                |    17 +-
 41 files changed, 25196 insertions(+), 172 deletions(-)
 create mode 100644 R/DFOP.solution.R
 create mode 100644 R/FOMC.solution.R
 create mode 100644 R/HS.solution.R
 create mode 100644 R/SFO.solution.R
 create mode 100644 R/SFORB.solution.R
 create mode 100644 R/mkinresplot.R
 create mode 100644 R/mkinstart.R
 create mode 100644 inst/GUI/.RData
 create mode 100644 inst/GUI/.Rhistory
 create mode 100644 inst/GUI/gdf-test.R
 create mode 100644 inst/GUI/simple-Gtk.R
 create mode 100644 inst/GUI/simple.R
 create mode 100644 inst/GUI/test.R
 create mode 100644 inst/doc/Rplots.pdf
 create mode 100644 man/DFOP.solution.Rd
 create mode 100644 man/FOMC.solution.Rd
 create mode 100644 man/HS.solution.Rd
 create mode 100644 man/SFO.solution.Rd
 create mode 100644 man/SFORB.solution.Rd
 create mode 100644 man/mkinresplot.Rd
 create mode 100644 man/mkinstart.Rd

diff --git a/DESCRIPTION b/DESCRIPTION
index 7eabdf2..a2c760c 100644
--- a/DESCRIPTION
+++ b/DESCRIPTION
@@ -2,18 +2,19 @@ Package: mkin
 Type: Package
 Title: Routines for fitting kinetic models with one or more state
   variables to chemical degradation data
-Version: 0.7-6
-Date: 2010-06-09
-Author: Johannes Ranke
-Maintainer: Johannes Ranke <jranke@harlan.com>
-Description: Calculation routines based on the FOCUS Kinetics Report (2006). Includes 
-  a function for conveniently defining differential equation models, choice of
-  the optimisation methods made available by the FME package (default is a
-  Levenberg-Marquardt variant).
-Depends: FME
+Version: 0.8-11
+Date: 2011-05-19
+Author: Johannes Ranke, Katrin Lindenberger
+Maintainer: Johannes Ranke <jranke@users.berlios.de>
+Description: Calculation routines based on the FOCUS Kinetics Report (2006).
+  Includes a function for conveniently defining differential equation models,
+  model solution based on eigenvalues if possible or using numerical solvers
+  and a choice of the optimisation methods made available by the FME package
+  (default is a Levenberg-Marquardt variant).  Please note that no warranty is
+  implied for correctness of results or fitness for a particular purpose.
+Depends: FME, deSolve, kinfit
+Suggests: RUnit
 License: GPL
 LazyLoad: yes
 LazyData: yes
-Packaged: 2010-05-18 12:52:36 UTC; ranke
-Repository: CRAN
-Date/Publication: 2010-05-18 13:18:05
+URL: http://cran.r-project.org, http://developer.berlios.de/projects/mkin/
diff --git a/R/DFOP.solution.R b/R/DFOP.solution.R
new file mode 100644
index 0000000..8531cfe
--- /dev/null
+++ b/R/DFOP.solution.R
@@ -0,0 +1,5 @@
+DFOP.solution <- function(t, parent.0, k1, k2, g)
+{
+	parent = g * parent.0 * exp(-k1 * t) +
+		 (1 - g) * parent.0 * exp(-k2 * t)
+}
diff --git a/R/FOMC.solution.R b/R/FOMC.solution.R
new file mode 100644
index 0000000..8bd13d6
--- /dev/null
+++ b/R/FOMC.solution.R
@@ -0,0 +1,4 @@
+FOMC.solution <- function(t, parent.0, alpha, beta)
+{
+	parent = parent.0 / (t/beta + 1)^alpha
+}
diff --git a/R/HS.solution.R b/R/HS.solution.R
new file mode 100644
index 0000000..4651a6a
--- /dev/null
+++ b/R/HS.solution.R
@@ -0,0 +1,6 @@
+HS.solution <- function(t, parent.0, k1, k2, tb)
+{
+	parent = ifelse(t <= tb, 
+		parent.0 * exp(-k1 * t),
+		parent.0 * exp(-k1 * tb) * exp(-k2 * (t - tb)))
+}
diff --git a/R/SFO.solution.R b/R/SFO.solution.R
new file mode 100644
index 0000000..3a376e4
--- /dev/null
+++ b/R/SFO.solution.R
@@ -0,0 +1,4 @@
+SFO.solution <- function(t, parent.0, k)
+{
+	parent = parent.0 * exp(-k * t)
+}
diff --git a/R/SFORB.solution.R b/R/SFORB.solution.R
new file mode 100644
index 0000000..45a4533
--- /dev/null
+++ b/R/SFORB.solution.R
@@ -0,0 +1,9 @@
+SFORB.solution = function(t, parent.0, k_12, k_21, k_1output) {
+  sqrt_exp = sqrt(1/4 * (k_12 + k_21 + k_1output)^2 + k_12 * k_21 - (k_12 + k_1output) * k_21)
+  b1 = 0.5 * (k_12 + k_21 + k_1output) + sqrt_exp
+  b2 = 0.5 * (k_12 + k_21 + k_1output) - sqrt_exp
+  
+  parent = parent.0 * 
+        (((k_12 + k_21 - b1)/(b2 - b1)) * exp(-b1 * t) +
+        ((k_12 + k_21 - b2)/(b1 - b2)) * exp(-b2 * t))
+}
diff --git a/R/mkin_long_to_wide.R b/R/mkin_long_to_wide.R
index 45ee0a1..ca09b49 100644
--- a/R/mkin_long_to_wide.R
+++ b/R/mkin_long_to_wide.R
@@ -1,7 +1,28 @@
-mkin_long_to_wide <- function(long_data, time = "time")
+# $Id: mkin_long_to_wide.R 96 2011-04-29 11:10:40Z jranke $
+
+# Copyright (C) 2010-2011 Johannes Ranke
+# Contact: mkin-devel@lists.berlios.de
+
+# This file is part of the R package mkin
+
+# mkin is free software: you can redistribute it and/or modify it under the
+# terms of the GNU General Public License as published by the Free Software
+# Foundation, either version 3 of the License, or (at your option) any later
+# version.
+
+# This program is distributed in the hope that it will be useful, but WITHOUT
+# ANY WARRANTY; without even the implied warranty of MERCHANTABILITY or FITNESS
+# FOR A PARTICULAR PURPOSE.  See the GNU General Public License for more
+# details.
+
+# You should have received a copy of the GNU General Public License along with
+# this program. If not, see <http://www.gnu.org/licenses/>
+
+mkin_long_to_wide <- function(long_data, time = "time", outtime = "time")
 {
   colnames <- unique(long_data$name)
   wide_data <- data.frame(time = subset(long_data, name == colnames[1], time))
+  names(wide_data) <- outtime
   for (var in colnames) {
     wide_data[var] <- subset(long_data, name == var, value)
   }
diff --git a/R/mkin_wide_to_long.R b/R/mkin_wide_to_long.R
index 21ab77b..995a9be 100644
--- a/R/mkin_wide_to_long.R
+++ b/R/mkin_wide_to_long.R
@@ -1,3 +1,23 @@
+# $Id: mkin_wide_to_long.R 59 2010-07-28 12:29:15Z jranke $
+
+# Copyright (C) 2010 Johannes Ranke
+# Contact: mkin-devel@lists.berlios.de
+
+# This file is part of the R package mkin
+
+# mkin is free software: you can redistribute it and/or modify it under the
+# terms of the GNU General Public License as published by the Free Software
+# Foundation, either version 3 of the License, or (at your option) any later
+# version.
+
+# This program is distributed in the hope that it will be useful, but WITHOUT
+# ANY WARRANTY; without even the implied warranty of MERCHANTABILITY or FITNESS
+# FOR A PARTICULAR PURPOSE.  See the GNU General Public License for more
+# details.
+
+# You should have received a copy of the GNU General Public License along with
+# this program. If not, see <http://www.gnu.org/licenses/>
+
 mkin_wide_to_long <- function(wide_data, time = "t")
 {
   colnames <- names(wide_data)
diff --git a/R/mkinerrmin.R b/R/mkinerrmin.R
index 7a922eb..ebed191 100644
--- a/R/mkinerrmin.R
+++ b/R/mkinerrmin.R
@@ -1,3 +1,23 @@
+# $Id: mkinerrmin.R 59 2010-07-28 12:29:15Z jranke $
+
+# Copyright (C) 2010 Johannes Ranke
+# Contact: mkin-devel@lists.berlios.de
+
+# This file is part of the R package mkin
+
+# mkin is free software: you can redistribute it and/or modify it under the
+# terms of the GNU General Public License as published by the Free Software
+# Foundation, either version 3 of the License, or (at your option) any later
+# version.
+
+# This program is distributed in the hope that it will be useful, but WITHOUT
+# ANY WARRANTY; without even the implied warranty of MERCHANTABILITY or FITNESS
+# FOR A PARTICULAR PURPOSE.  See the GNU General Public License for more
+# details.
+
+# You should have received a copy of the GNU General Public License along with
+# this program. If not, see <http://www.gnu.org/licenses/>
+
 mkinerrmin <- function(errdata, n.parms, alpha = 0.05)
 {
   means.mean <- mean(errdata$value_mean, na.rm=TRUE)
diff --git a/R/mkinfit.R b/R/mkinfit.R
index f8285fc..b742742 100644
--- a/R/mkinfit.R
+++ b/R/mkinfit.R
@@ -1,11 +1,36 @@
+# $Id: mkinfit.R 120 2011-09-02 14:25:35Z jranke $
+
+# Copyright (C) 2010-2011 Johannes Ranke
+# Contact: mkin-devel@lists.berlios.de
+# The summary function is an adapted and extended version of summary.modFit
+# from the FME package, v 1.1 by Soetart and Petzoldt, which was in turn
+# inspired by summary.nls.lm
+
+# This file is part of the R package mkin
+
+# mkin is free software: you can redistribute it and/or modify it under the
+# terms of the GNU General Public License as published by the Free Software
+# Foundation, either version 3 of the License, or (at your option) any later
+# version.
+
+# This program is distributed in the hope that it will be useful, but WITHOUT
+# ANY WARRANTY; without even the implied warranty of MERCHANTABILITY or FITNESS
+# FOR A PARTICULAR PURPOSE.  See the GNU General Public License for more
+# details.
+
+# You should have received a copy of the GNU General Public License along with
+# this program. If not, see <http://www.gnu.org/licenses/>
+
 mkinfit <- function(mkinmod, observed,
   parms.ini = rep(0.1, length(mkinmod$parms)),
   state.ini = c(100, rep(0, length(mkinmod$diffs) - 1)), 
   lower = 0, upper = Inf,
   fixed_parms = NULL,
   fixed_initials = names(mkinmod$diffs)[-1],
+  eigen = FALSE,
   plot = FALSE, quiet = FALSE,
   err = NULL, weight = "none", scaleVar = FALSE,
+  atol = 1e-6,
   ...)
 {
   mod_vars <- names(mkinmod$diffs)
@@ -16,18 +41,6 @@ mkinfit <- function(mkinmod, observed,
 
   # Name the parameters if they are not named yet
   if(is.null(names(parms.ini))) names(parms.ini) <- mkinmod$parms
-  # Create a function calculating the differentials specified by the model
-  mkindiff <- function(t, state, parms) {
-    time <- t
-    diffs <- vector()
-    for (box in mod_vars)
-    {
-      diffname <- paste("d", box, sep="_")      
-      diffs[diffname] <- with(as.list(c(time,state, parms)),
-        eval(parse(text=mkinmod$diffs[[box]])))
-    }
-    return(list(c(diffs)))
-  } 
 
   # Name the inital parameter values if they are not named yet
   if(is.null(names(state.ini))) names(state.ini) <- mod_vars
@@ -45,6 +58,40 @@ mkinfit <- function(mkinmod, observed,
       names(state.ini.optim) <- paste(names(state.ini.optim), "0", sep="_")
   }
 
+  # Set upper limit for formation fractions to one if formation fractions are
+  # directly defined and if no user input for upper limit is given
+  if (all(upper==Inf) & any(grepl("f_", names(parms.ini)))==TRUE){
+    upper=c( rep(Inf,length(parms.optim)))
+    upper[grep("f_", names(parms.optim))]=1
+    upper=c(rep(Inf, length(state.ini.optim)), upper)
+  }
+
+  # Decide if the solution of the model can be based on a simple analytical
+  # formula, the spectral decomposition of the matrix (fundamental system)
+  # or a numeric ode solver from the deSolve package
+  if (length(mkinmod$map) == 1) {
+    solution = "analytical"
+  } else {
+    if (is.matrix(mkinmod$coefmat) & eigen) solution = "eigen"
+    else solution = "deSolve"
+  }
+
+  # Create a function calculating the differentials specified by the model
+  # if necessary
+  if(solution == "deSolve") {
+    mkindiff <- function(t, state, parms) {
+      time <- t
+      diffs <- vector()
+      for (box in mod_vars)
+      {
+        diffname <- paste("d", box, sep="_")      
+        diffs[diffname] <- with(as.list(c(time,state, parms)),
+          eval(parse(text=mkinmod$diffs[[box]])))
+      }
+      return(list(c(diffs)))
+    } 
+  }
+
   cost.old <- 1e100
   calls <- 0
   out_predicted <- NA
@@ -60,19 +107,67 @@ mkinfit <- function(mkinmod, observed,
     odeparms <- c(P[(length(state.ini.optim) + 1):length(P)], parms.fixed)
 
     outtimes = unique(observed$time)
+    evalparse <- function(string)
+    {
+      eval(parse(text=string), as.list(c(odeparms, odeini)))
+    }
 
-    # Solve the ode
-    out <- ode(
-      y = odeini,
-      times = outtimes,
-      func = mkindiff, 
-      parms = odeparms)
-
+    # Solve the system
+    if (solution == "analytical") {
+      parent.type = names(mkinmod$map[[1]])[1]  
+      parent.name = names(mkinmod$diffs)[[1]]
+      o <- switch(parent.type,
+        SFO = SFO.solution(outtimes, 
+            evalparse(parent.name),
+            evalparse(paste("k", parent.name, "sink", sep="_"))),
+        FOMC = FOMC.solution(outtimes,
+            evalparse(parent.name),
+            evalparse("alpha"), evalparse("beta")),
+        DFOP = DFOP.solution(outtimes,
+            evalparse(parent.name),
+            evalparse("k1"), evalparse("k2"),
+            evalparse("g")),
+        HS = HS.solution(outtimes,
+            evalparse(parent.name),
+            evalparse("k1"), evalparse("k2"),
+            evalparse("tb")),
+        SFORB = SFORB.solution(outtimes,
+            evalparse(parent.name),
+            evalparse(paste("k", parent.name, "bound", sep="_")),
+            evalparse(paste("k", sub("free", "bound", parent.name), "free", sep="_")),
+            evalparse(paste("k", parent.name, "sink", sep="_")))
+      )
+      out <- cbind(outtimes, o)
+      dimnames(out) <- list(outtimes, c("time", sub("_free", "", parent.name)))
+    }
+    if (solution == "eigen") {
+      coefmat.num <- matrix(sapply(as.vector(mkinmod$coefmat), evalparse), 
+        nrow = length(mod_vars))
+      e <- eigen(coefmat.num)
+      c <- solve(e$vectors, odeini)
+      f.out <- function(t) {
+        e$vectors %*% diag(exp(e$values * t), nrow=length(mod_vars)) %*% c
+      }
+      o <- matrix(mapply(f.out, outtimes), 
+        nrow = length(mod_vars), ncol = length(outtimes))
+      dimnames(o) <- list(mod_vars, outtimes)
+      out <- cbind(time = outtimes, t(o))
+    } 
+    if (solution == "deSolve")  
+    {
+      out <- ode(
+        y = odeini,
+        times = outtimes,
+        func = mkindiff, 
+        parms = odeparms,
+        atol = atol
+      )
+    }
   
     # Output transformation for models with unobserved compartments like SFORB
     out_transformed <- data.frame(time = out[,"time"])
     for (var in names(mkinmod$map)) {
-      if(length(mkinmod$map[[var]]) == 1) {
+      if((length(mkinmod$map[[var]]) == 1) || solution == "analytical") {
         out_transformed[var] <- out[, var]
       } else {
         out_transformed[var] <- rowSums(out[, mkinmod$map[[var]]])
@@ -90,19 +185,53 @@ mkinfit <- function(mkinmod, observed,
       # Plot the data and current model output if requested
       if(plot) {
         outtimes_plot = seq(min(observed$time), max(observed$time), length.out=100)
-        out_plot <- ode(
-          y = odeini,
-          times = outtimes_plot,
-          func = mkindiff, 
-          parms = odeparms)
+        if (solution == "analytical") {
+          o_plot <- switch(parent.type,
+            SFO = SFO.solution(outtimes_plot, 
+                evalparse(parent.name),
+                evalparse(paste("k", parent.name, "sink", sep="_"))),
+            FOMC = FOMC.solution(outtimes_plot,
+                evalparse(parent.name),
+                evalparse("alpha"), evalparse("beta")),
+            DFOP = DFOP.solution(outtimes_plot,
+                evalparse(parent.name),
+                evalparse("k1"), evalparse("k2"),
+                evalparse("g")),
+            HS = HS.solution(outtimes_plot,
+                evalparse(parent.name),
+                evalparse("k1"), evalparse("k2"),
+                evalparse("tb")),
+            SFORB = SFORB.solution(outtimes_plot,
+                evalparse(parent.name),
+                evalparse(paste("k", parent.name, "bound", sep="_")),
+                evalparse(paste("k", sub("free", "bound", parent.name), "free", sep="_")),
+                evalparse(paste("k", parent.name, "sink", sep="_")))
+          )
+          out_plot <- cbind(outtimes_plot, o_plot)
+          dimnames(out_plot) <- list(outtimes_plot, c("time", sub("_free", "", parent.name)))
+        }
+        if(solution == "eigen") {
+          o_plot <- matrix(mapply(f.out, outtimes_plot), 
+            nrow = length(mod_vars), ncol = length(outtimes_plot))
+          dimnames(o_plot) <- list(mod_vars, outtimes_plot)
+          out_plot <- cbind(time = outtimes_plot, t(o_plot))
+        } 
+        if (solution == "deSolve") {
+          out_plot <- ode(
+            y = odeini,
+            times = outtimes_plot,
+            func = mkindiff, 
+            parms = odeparms)
+        }
         out_transformed_plot <- data.frame(time = out_plot[,"time"])
-        for (var in names(mkinmod$map)) {
-          if(length(mkinmod$map[[var]]) == 1) {
+        for (var in obs_vars) {
+          if((length(mkinmod$map[[var]]) == 1) || solution == "analytical") {
             out_transformed_plot[var] <- out_plot[, var]
           } else {
             out_transformed_plot[var] <- rowSums(out_plot[, mkinmod$map[[var]]])
           }
         }    
+        out_transformed_plot <<- out_transformed_plot
 
         plot(0, type="n", 
           xlim = range(observed$time), ylim = range(observed$value, na.rm=TRUE),
@@ -124,8 +253,17 @@ mkinfit <- function(mkinmod, observed,
   }
   fit <- modFit(cost, c(state.ini.optim, parms.optim), lower = lower, upper = upper, ...)
 
-  # We need the function for plotting
-  fit$mkindiff <- mkindiff
+  # We need to return some more data for summary and plotting
+  fit$solution <- solution
+  if (solution == "eigen") {
+    fit$coefmat <- mkinmod$coefmat
+  } 
+  if (solution == "deSolve") {
+    fit$mkindiff <- mkindiff
+  }
+  if (plot == TRUE) {
+    fit$out_transformed_plot = out_transformed_plot
+  }
 
   # We also need various other information for summary and plotting
   fit$map <- mkinmod$map
@@ -161,54 +299,109 @@ mkinfit <- function(mkinmod, observed,
     n.optim <- n.k.optim + n.initials.optim
     if ("alpha" %in% names(parms.optim)) n.optim <- n.optim + 1
     if ("beta" %in% names(parms.optim)) n.optim <- n.optim + 1
+    if ("k1" %in% names(parms.optim)) n.optim <- n.optim + 1
+    if ("k2" %in% names(parms.optim)) n.optim <- n.optim + 1
+    if ("g" %in% names(parms.optim)) n.optim <- n.optim + 1
+    if ("tb" %in% names(parms.optim)) n.optim <- n.optim + 1
     errmin.tmp <- mkinerrmin(errdata.var, n.optim)
     errmin[obs_var, c("err.min", "n.optim", "df")] <- errmin.tmp
   }
   fit$errmin <- errmin
 
-  # Calculate dissipation times DT50 and DT90
+  # Calculate dissipation times DT50 and DT90 and formation fractions
   parms.all = c(fit$par, parms.fixed)
   fit$distimes <- data.frame(DT50 = rep(NA, length(obs_vars)), DT90 = rep(NA, length(obs_vars)), 
     row.names = obs_vars)
+  fit$ff <- vector()
+  fit$SFORB <- vector()
   for (obs_var in obs_vars) {
-      type = names(mkinmod$map[[obs_var]])[1]  
-      if (type == "SFO") {
-        k_names = grep(paste("k", obs_var, sep="_"), names(parms.all), value=TRUE)
-        k_tot = sum(parms.all[k_names])
-        DT50 = log(2)/k_tot
-        DT90 = log(10)/k_tot
+    type = names(mkinmod$map[[obs_var]])[1]  
+    if (type == "SFO") {
+      k_names = grep(paste("k", obs_var, sep="_"), names(parms.all), value=TRUE)
+      k_tot = sum(parms.all[k_names])
+      DT50 = log(2)/k_tot
+      DT90 = log(10)/k_tot
+      for (k_name in k_names)
+      {
+        fit$ff[[sub("k_", "", k_name)]] = parms.all[[k_name]] / k_tot
       }
-      if (type == "FOMC") {
-        alpha = parms.all["alpha"]
-        beta = parms.all["beta"]
-        DT50 = beta * (2^(1/alpha) - 1)
-        DT90 = beta * (10^(1/alpha) - 1)
+    }
+    if (type == "FOMC") {
+      alpha = parms.all["alpha"]
+      beta = parms.all["beta"]
+      DT50 = beta * (2^(1/alpha) - 1)
+      DT90 = beta * (10^(1/alpha) - 1)
+    }
+    if (type == "DFOP") {
+      k1 = parms.all["k1"]
+      k2 = parms.all["k2"]
+      g = parms.all["g"]
+      f <- function(t, x) {
+        fraction <- g * exp( - k1 * t) + (1 - g) * exp( - k2 * t)
+        (fraction - (1 - x/100))^2
       }
-      if (type == "SFORB") {
-        # FOCUS kinetics (2006), p. 60 f
-        k_out_names = grep(paste("k", obs_var, "free", sep="_"), names(parms.all), value=TRUE)
-        k_out_names = setdiff(k_out_names, paste("k", obs_var, "free", "bound", sep="_"))
-        k_1output = sum(parms.all[k_out_names])
-        k_12 = parms.all[paste("k", obs_var, "free", "bound", sep="_")]
-        k_21 = parms.all[paste("k", obs_var, "bound", "free", sep="_")]
-
-        sqrt_exp = sqrt(1/4 * (k_12 + k_21 + k_1output)^2 + k_12 * k_21 - (k_12 + k_1output) * k_21)
-        b1 = 0.5 * (k_12 + k_21 + k_1output) + sqrt_exp
-        b2 = 0.5 * (k_12 + k_21 + k_1output) - sqrt_exp
-
-        SFORB_fraction = function(t) {
-          ((k_12 + k_21 - b1)/(b2 - b1)) * exp(-b1 * t) +
-          ((k_12 + k_21 - b2)/(b1 - b2)) * exp(-b2 * t)
-        }
-        f_50 <- function(t) (SFORB_fraction(t) - 0.5)^2
-        max_DT <- 1000
-        DT50.o <- optimize(f_50, c(0.01, max_DT))$minimum
-        if (abs(DT50.o - max_DT) < 0.01) DT50 = NA else DT50 = DT50.o
-        f_90 <- function(t) (SFORB_fraction(t) - 0.1)^2
-        DT90.o <- optimize(f_90, c(0.01, 1000))$minimum
-        if (abs(DT90.o - max_DT) < 0.01) DT90 = NA else DT90 = DT90.o
+      DTmax <- 1000
+      DT50.o <- optimize(f, c(0.001, DTmax), x=50)$minimum
+      DT50 = ifelse(DTmax - DT50.o < 0.1, NA, DT50.o)
+      DT90.o <- optimize(f, c(0.001, DTmax), x=90)$minimum
+      DT90 = ifelse(DTmax - DT90.o < 0.1, NA, DT90.o)
+    }
+    if (type == "HS") {
+      k1 = parms.all["k1"]
+      k2 = parms.all["k2"]
+      tb = parms.all["tb"]
+      DTx <- function(x) {
+        DTx.a <- (log(100/(100 - x)))/k1
+        DTx.b <- tb + (log(100/(100 - x)) - k1 * tb)/k2
+        if (DTx.a < tb) DTx <- DTx.a
+        else DTx <- DTx.b
+        return(DTx)
       }
-      fit$distimes[obs_var, ] = c(DT50, DT90)
+      DT50 <- DTx(50)
+      DT90 <- DTx(90)
+    }
+    # Back-calculation of formation fractions in case of nonlinear parent kinetics
+    if (type %in% c("FOMC", "DFOP", "HS")) {
+      ff_names = names(mkinmod$ff)
+      for (ff_name in ff_names)
+      {
+        fit$ff[[paste(obs_var, ff_name, sep="_")]] = 
+          eval(parse(text = mkinmod$ff[ff_name]), as.list(parms.all))
+      }
+      fit$ff[[paste(obs_var, "sink", sep="_")]] = 1 - sum(fit$ff)
+    }
+    if (type == "SFORB") {
+      # FOCUS kinetics (2006), p. 60 f
+      k_out_names = grep(paste("k", obs_var, "free", sep="_"), names(parms.all), value=TRUE)
+      k_out_names = setdiff(k_out_names, paste("k", obs_var, "free", "bound", sep="_"))
+      k_1output = sum(parms.all[k_out_names])
+      k_12 = parms.all[paste("k", obs_var, "free", "bound", sep="_")]
+      k_21 = parms.all[paste("k", obs_var, "bound", "free", sep="_")]
+
+      sqrt_exp = sqrt(1/4 * (k_12 + k_21 + k_1output)^2 + k_12 * k_21 - (k_12 + k_1output) * k_21)
+      b1 = 0.5 * (k_12 + k_21 + k_1output) + sqrt_exp
+      b2 = 0.5 * (k_12 + k_21 + k_1output) - sqrt_exp
+
+      SFORB_fraction = function(t) {
+        ((k_12 + k_21 - b1)/(b2 - b1)) * exp(-b1 * t) +
+        ((k_12 + k_21 - b2)/(b1 - b2)) * exp(-b2 * t)
+      }
+      f_50 <- function(t) (SFORB_fraction(t) - 0.5)^2
+      max_DT <- 1000
+      DT50.o <- optimize(f_50, c(0.01, max_DT))$minimum
+      if (abs(DT50.o - max_DT) < 0.01) DT50 = NA else DT50 = DT50.o
+      f_90 <- function(t) (SFORB_fraction(t) - 0.1)^2
+      DT90.o <- optimize(f_90, c(0.01, max_DT))$minimum
+      if (abs(DT90.o - max_DT) < 0.01) DT90 = NA else DT90 = DT90.o
+      for (k_out_name in k_out_names)
+      {
+        fit$ff[[sub("k_", "", k_out_name)]] = parms.all[[k_out_name]] / k_1output
+      }
+      # Return the eigenvalues for comparison with DFOP rate constants
+      fit$SFORB[[paste(obs_var, "b1", sep="_")]] = b1
+      fit$SFORB[[paste(obs_var, "b2", sep="_")]] = b2
+    }
+    fit$distimes[obs_var, ] = c(DT50, DT90)
   }
 
   # Collect observed, predicted and residuals
@@ -217,25 +410,74 @@ mkinfit <- function(mkinmod, observed,
   data$residual <- data$observed - data$predicted
   data$variable <- ordered(data$variable, levels = obs_vars)
   fit$data <- data[order(data$variable, data$time), ]
+  fit$atol <- atol
 
   class(fit) <- c("mkinfit", "modFit") 
   return(fit)
 }
 
-summary.mkinfit <- function(object, data = TRUE, distimes = TRUE, cov = FALSE,...) {
-  ans <- FME:::summary.modFit(object, cov = cov)
+summary.mkinfit <- function(object, data = TRUE, distimes = TRUE, ff = TRUE, cov = FALSE,...) {
+  param  <- object$par
+  pnames <- names(param)
+  p      <- length(param)
+  covar  <- try(solve(0.5*object$hessian), silent = TRUE)   # unscaled covariance
+  if (!is.numeric(covar)) {
+    message <- "Cannot estimate covariance; system is singular"
+    warning(message)
+    covar <- matrix(data = NA, nrow = p, ncol = p)
+  } else message <- "ok"
+
+  rownames(covar) <- colnames(covar) <-pnames
+  rdf    <- object$df.residual
+  resvar <- object$ssr / rdf
+  se     <- sqrt(diag(covar) * resvar)
+  names(se) <- pnames
+  tval      <- param / se
+  modVariance <- object$ssr / length(object$residuals)
+
+  if (!all(object$start$lower >=0)) {
+    message <- "Note that the one-sided t-test may not be appropriate if
+      parameter values below zero are possible."
+    warning(message)
+  } else message <- "ok"
+
+  param <- cbind(param, se, tval, pt(tval, rdf, lower.tail = FALSE))
+  dimnames(param) <- list(pnames, c("Estimate", "Std. Error",
+                                    "t value", "Pr(>t)"))
+  if(cov)
+    ans <- list(residuals = object$residuals,
+                residualVariance = resvar,
+                sigma = sqrt(resvar),
+                modVariance = modVariance,
+                df = c(p, rdf), cov.unscaled = covar,
+                cov.scaled = covar * resvar,
+                info = object$info, niter = object$iterations,
+                stopmess = message,
+                par = param)
+  else
+    ans <- list(residuals = object$residuals,
+                residualVariance = resvar,
+                sigma = sqrt(resvar),
+                modVariance = modVariance,
+                df = c(p, rdf),
+                info = object$info, niter = object$iterations,
+                stopmess = message,
+                par = param)
+
   ans$diffs <- object$diffs
   if(data) ans$data <- object$data
   ans$start <- object$start
   ans$fixed <- object$fixed
   ans$errmin <- object$errmin 
   if(distimes) ans$distimes <- object$distimes
+  if(ff) ans$ff <- object$ff
+  if(length(object$SFORB) != 0) ans$SFORB <- object$SFORB
   class(ans) <- c("summary.mkinfit", "summary.modFit") 
   return(ans)  
 }
 
 # Expanded from print.summary.modFit
-print.summary.mkinfit <- function(x, digits = max(3, getOption("digits") - 3), ...) {
+print.summary.mkinfit <- function(x, digits = max(3, getOption("digits") - 3), tval = TRUE, ...) {
   cat("\nEquations:\n")
   print(noquote(as.character(x[["diffs"]])))
   df  <- x$df
@@ -249,7 +491,11 @@ print.summary.mkinfit <- function(x, digits = max(3, getOption("digits") - 3), .
   else print(x$fixed)
   
   cat("\nOptimised parameters:\n")
-  printCoefmat(x$par, digits = digits, ...)
+  if (tval) printCoefmat(x$par, digits = digits, ...)
+  else {
+    printCoefmat(x$par[,c(1,2,4)], cs.in = c(1,2), tst.ind = integer(0), 
+      P.values = TRUE, has.Pvalue = TRUE, digits = digits, ...)
+  }
 
   cat("\nResidual standard error:",
       format(signif(x$sigma, digits)), "on", rdf, "degrees of freedom\n")
@@ -260,10 +506,22 @@ print.summary.mkinfit <- function(x, digits = max(3, getOption("digits") - 3), .
 
   printdistimes <- !is.null(x$distimes)
   if(printdistimes){
-    cat("\nEstimated disappearance times\n")
+    cat("\nEstimated disappearance times:\n")
     print(x$distimes, digits=digits,...)
   }    
 
+  printff <- !is.null(x$ff)
+  if(printff){
+    cat("\nEstimated formation fractions:\n")
+    print(data.frame(ff = x$ff), digits=digits,...)
+  }    
+
+  printSFORB <- !is.null(x$SFORB)
+  if(printSFORB){
+    cat("\nEstimated Eigenvalues of SFORB model(s):\n")
+    print(x$SFORB, digits=digits,...)
+  }    
+
   printcor <- !is.null(x$cov.unscaled)
   if (printcor){
     Corr <- cov2cor(x$cov.unscaled)
diff --git a/R/mkinmod.R b/R/mkinmod.R
index 643e855..31c778c 100644
--- a/R/mkinmod.R
+++ b/R/mkinmod.R
@@ -1,3 +1,23 @@
+# $Id: mkinmod.R 71 2010-09-12 01:13:36Z jranke $
+
+# Copyright (C) 2010 Johannes Ranke
+# Contact: mkin-devel@lists.berlios.de
+
+# This file is part of the R package mkin
+
+# mkin is free software: you can redistribute it and/or modify it under the
+# terms of the GNU General Public License as published by the Free Software
+# Foundation, either version 3 of the License, or (at your option) any later
+# version.
+
+# This program is distributed in the hope that it will be useful, but WITHOUT
+# ANY WARRANTY; without even the implied warranty of MERCHANTABILITY or FITNESS
+# FOR A PARTICULAR PURPOSE.  See the GNU General Public License for more
+# details.
+
+# You should have received a copy of the GNU General Public License along with
+# this program. If not, see <http://www.gnu.org/licenses/>
+
 mkinmod <- function(...)
 {
   spec <- list(...)
@@ -5,22 +25,36 @@ mkinmod <- function(...)
 
   # The returned model will be a list of character vectors, containing
   # differential equations, parameter names and a mapping from model variables
-  # to observed variables
+  # to observed variables. If possible, a matrix representation of the 
+  # differential equations is included
   parms <- vector()
   diffs <- vector()
   map <- list()
+  if(spec[[1]]$type %in% c("FOMC", "DFOP", "HS")) {
+    mat = FALSE 
+    if(!is.null(spec[[1]]$to)) {
+      message <- paste("Only constant formation fractions over time are implemented.",
+        "Depending on the reason for the time dependence of degradation, this may be unrealistic",
+        sep="\n")
+      warning(message)
+    } else message <- "ok"
+  } else mat = TRUE
 
   # Establish list of differential equations
   for (varname in obs_vars)
   {
-    if(is.null(spec[[varname]]$type)) stop("Every argument to mkinmod must be a list containing a type component")
-    if(!spec[[varname]]$type %in% c("SFO", "FOMC", "SFORB")) stop("Available types are SFO, FOMC and SFORB only")
+    if(is.null(spec[[varname]]$type)) stop(
+      "Every argument to mkinmod must be a list containing a type component")
+    if(!spec[[varname]]$type %in% c("SFO", "FOMC", "DFOP", "HS", "SFORB")) stop(
+      "Available types are SFO, FOMC, DFOP, HS and SFORB only")
     new_parms <- vector()
 
     # New (sub)compartments (boxes) needed for the model type
     new_boxes <- switch(spec[[varname]]$type,
       SFO = varname,
       FOMC = varname,
+      DFOP = varname,
+      HS = varname,
       SFORB = paste(varname, c("free", "bound"), sep="_")
     )
     map[[varname]] <- new_boxes
@@ -29,25 +63,64 @@ mkinmod <- function(...)
     # Start a new differential equation for each new box
     new_diffs <- paste("d_", new_boxes, " =", sep="")
 
-    # Construct terms for transfer to sink and add if appropriate
+    # Turn on sink if not specified otherwise
     if(is.null(spec[[varname]]$sink)) spec[[varname]]$sink <- TRUE
+
+    # Construct and add FOMC term and add FOMC parameters if needed
+    if(spec[[varname]]$type == "FOMC") {
+      if(match(varname, obs_vars) != 1) {
+        stop("Type FOMC is only possible for the first compartment, which is assumed to be the source compartment")
+      }
+      if(spec[[varname]]$sink == FALSE) {
+        stop("Turning off the sink for the FOMC model is not implemented")
+      }
+      # From p. 53 of the FOCUS kinetics report
+      nonlinear_term <- paste("(alpha/beta) * ((time/beta) + 1)^-1 *", new_boxes[[1]])
+      new_diffs[[1]] <- paste(new_diffs[[1]], "-", nonlinear_term)
+      new_parms <- c("alpha", "beta")
+      ff <- vector()
+    } 
+
+    # Construct and add DFOP term and add DFOP parameters if needed
+    if(spec[[varname]]$type == "DFOP") {
+      if(match(varname, obs_vars) != 1) {
+        stop("Type DFOP is only possible for the first compartment, which is assumed to be the source compartment")
+      }
+      if(spec[[varname]]$sink == FALSE) {
+        stop("Turning off the sink for the DFOP model is not implemented")
+      }
+      # From p. 57 of the FOCUS kinetics report
+      nonlinear_term <- paste("((k1 * g * exp(-k1 * time) + k2 * (1 - g) * exp(-k2 * time)) / (g * exp(-k1 * time) + (1 - g) * exp(-k2 * time))) *", new_boxes[[1]])
+      new_diffs[[1]] <- paste(new_diffs[[1]], "-", nonlinear_term)
+      new_parms <- c("k1", "k2", "g")
+      ff <- vector()
+    } 
+
+    # Construct and add HS term and add HS parameters if needed
+    if(spec[[varname]]$type == "HS") {
+      if(match(varname, obs_vars) != 1) {
+        stop("Type HS is only possible for the first compartment, which is assumed to be the source compartment")
+      }
+      if(spec[[varname]]$sink == FALSE) {
+        stop("Turning off the sink for the HS model is not implemented")
+      }
+      # From p. 55 of the FOCUS kinetics report
+      nonlinear_term <- paste("ifelse(time <= tb, k1, k2)", "*", new_boxes[[1]])
+      new_diffs[[1]] <- paste(new_diffs[[1]], "-", nonlinear_term)
+      new_parms <- c("k1", "k2", "tb")
+      ff <- vector()
+    } 
+
+    # Construct terms for transfer to sink and add if appropriate
+
     if(spec[[varname]]$sink) {
-      # Add first-order sink term to first (or only) box for SFO and SFORB models
+      # Add first-order sink term to first (or only) box for SFO and SFORB
       if(spec[[varname]]$type %in% c("SFO", "SFORB")) {
         k_compound_sink <- paste("k", new_boxes[[1]], "sink", sep="_")
         sink_term <- paste("-", k_compound_sink, "*", new_boxes[[1]])
         new_diffs[[1]] <- paste(new_diffs[[1]], sink_term)
         new_parms <- k_compound_sink
       }
-      if(spec[[varname]]$type == "FOMC") {
-        if(match(varname, obs_vars) != 1) {
-          stop("Type FOMC is only allowed for the first compartment, which is assumed to be the source compartment")
-        }
-        # From p. 53 of the FOCUS kinetics report
-        fomc_term <- paste("(alpha/beta) * ((time/beta) + 1)^-1 *", new_boxes[[1]])
-        new_diffs[[1]] <- paste(new_diffs[[1]], "-", fomc_term)
-        new_parms <- c("alpha", "beta")
-      }
     }
    
     # Add reversible binding if appropriate
@@ -66,7 +139,6 @@ mkinmod <- function(...)
     names(new_diffs) <- new_boxes
     diffs <- c(diffs, new_diffs)
   }
-
   # Transfer between compartments
   for (varname in obs_vars) {
     to <- spec[[varname]]$to
@@ -74,6 +146,8 @@ mkinmod <- function(...)
       origin_box <- switch(spec[[varname]]$type,
         SFO = varname,
         FOMC = varname,
+        DFOP = varname,
+        HS = varname,
         SFORB = paste(varname, "free", sep="_"))
       fraction_left <- NULL
       for (target in to) {
@@ -82,27 +156,63 @@ mkinmod <- function(...)
           SFORB = paste(target, "free", sep="_"))
         if(spec[[varname]]$type %in% c("SFO", "SFORB")) {
           k_from_to <- paste("k", origin_box, target_box, sep="_")
-          diffs[[origin_box]] <- paste(diffs[[origin_box]], "-", k_from_to, "*", origin_box)
-          diffs[[target_box]] <- paste(diffs[[target_box]], "+", k_from_to, "*", origin_box)
+          diffs[[origin_box]] <- paste(diffs[[origin_box]], "-", 
+            k_from_to, "*", origin_box)
+          diffs[[target_box]] <- paste(diffs[[target_box]], "+", 
+            k_from_to, "*", origin_box)
           parms <- c(parms, k_from_to)
         }
-        if(spec[[varname]]$type == "FOMC") {
+        if(spec[[varname]]$type %in% c("FOMC", "DFOP", "HS")) {
           fraction_to_target = paste("f_to", target, sep="_")
-          fraction_not_to_target = paste("(1 - ", fraction_to_target, ")", sep="")
+          fraction_not_to_target = paste("(1 - ", fraction_to_target, ")", 
+            sep="")
           if(is.null(fraction_left)) {
             fraction_really_to_target = fraction_to_target
             fraction_left = fraction_not_to_target
           } else {
-            fraction_really_to_target = paste(fraction_left, " * ", fraction_to_target, sep="")
-            fraction_left = paste(fraction_left, " * ", fraction_not_to_target, sep="")
+            fraction_really_to_target = paste(fraction_left, " * ", 
+              fraction_to_target, sep="")
+            fraction_left = paste(fraction_left, " * ", 
+              fraction_not_to_target, sep="")
           }
-          diffs[[target_box]] <- paste(diffs[[target_box]], "+", fraction_really_to_target, "*", fomc_term)
+          ff[target_box] = fraction_really_to_target
+          diffs[[target_box]] <- paste(diffs[[target_box]], "+", 
+            ff[target_box], "*", nonlinear_term)
           parms <- c(parms, fraction_to_target)
         }
       }
     }
   }
   model <- list(diffs = diffs, parms = parms, map = map)
+
+  # Create coefficient matrix if appropriate
+  if (mat) {
+    boxes <- names(diffs)
+    n <- length(boxes)
+    m <- matrix(nrow=n, ncol=n, dimnames=list(boxes, boxes))
+    for (from in boxes) {
+      for (to in boxes) {
+        if (from == to) {
+          k.candidate = paste("k", from, c(boxes, "sink"), sep="_")
+          k.candidate = sub("free.*bound", "free_bound", k.candidate)
+          k.candidate = sub("bound.*free", "bound_free", k.candidate)
+          k.effective = intersect(model$parms, k.candidate)
+          m[from,to] = ifelse(length(k.effective) > 0,
+              paste("-", k.effective, collapse = " "), "0")
+        } else {
+          k.candidate = paste("k", from, to, sep="_")
+          k.candidate = sub("free.*bound", "free_bound", k.candidate)
+          k.candidate = sub("bound.*free", "bound_free", k.candidate)
+          k.effective = intersect(model$parms, k.candidate)
+          m[to, from] = ifelse(length(k.effective) > 0,
+              k.effective, "0")
+        }
+      }
+    }
+    model$coefmat <- m
+  }
+
+  if (exists("ff")) model$ff = ff
   class(model) <- "mkinmod"
   invisible(model)
 }
diff --git a/R/mkinplot.R b/R/mkinplot.R
index d2880c0..d665bc2 100644
--- a/R/mkinplot.R
+++ b/R/mkinplot.R
@@ -1,5 +1,6 @@
-mkinplot <- function(fit, xlab = "Time", ylab = "Observed", xlim = range(fit$data$time), ylim = range(fit$data$observed, na.rm = TRUE), ...)
+mkinplot <- function(fit, xlab = "Time", ylab = "Observed", xlim = range(fit$data$time), ylim = range(fit$data$observed, na.rm = TRUE), legend = TRUE, ...)
 {
+  solution = fit$solution
   fixed <- fit$fixed$value
   names(fixed) <- rownames(fit$fixed)
   parms.all <- c(fit$par, fixed)
@@ -16,12 +17,60 @@ mkinplot <- function(fit, xlab = "Time", ylab = "Observed", xlim = range(fit$dat
     rownames(subset(fit$fixed, type == "deparm")))
   odeparms <- parms.all[odenames]
 
-  # Solve the ode
-  out <- ode(
-    y = odeini,
-    times = outtimes,
-    func = fit$mkindiff, 
-    parms = odeparms)
+  # Solve the system
+  evalparse <- function(string)
+  {
+    eval(parse(text=string), as.list(c(odeparms, odeini)))
+  }
+  if (solution == "analytical") {
+    parent.type = names(fit$map[[1]])[1]  
+    parent.name = names(fit$diffs)[[1]]
+    o <- switch(parent.type,
+      SFO = SFO.solution(outtimes, 
+          evalparse(parent.name),
+          evalparse(paste("k", parent.name, "sink", sep="_"))),
+      FOMC = FOMC.solution(outtimes,
+          evalparse(parent.name),
+          evalparse("alpha"), evalparse("beta")),
+      DFOP = DFOP.solution(outtimes,
+          evalparse(parent.name),
+          evalparse("k1"), evalparse("k2"),
+          evalparse("g")),
+      HS = HS.solution(outtimes,
+          evalparse(parent.name),
+          evalparse("k1"), evalparse("k2"),
+          evalparse("tb")),
+      SFORB = SFORB.solution(outtimes,
+          evalparse(parent.name),
+          evalparse(paste("k", parent.name, "free_bound", sep="_")),
+          evalparse(paste("k", parent.name, "bound_free", sep="_")),
+          evalparse(paste("k", parent.name, "free_sink", sep="_")))
+    )
+    out <- cbind(outtimes, o)
+    dimnames(out) <- list(outtimes, c("time", parent.name))
+  }
+  if (solution == "eigen") {
+    coefmat.num <- matrix(sapply(as.vector(fit$coefmat), evalparse), 
+      nrow = length(odeini))
+    e <- eigen(coefmat.num)
+    c <- solve(e$vectors, odeini)
+    f.out <- function(t) {
+      e$vectors %*% diag(exp(e$values * t), nrow=length(odeini)) %*% c
+    }
+    o <- matrix(mapply(f.out, outtimes), 
+      nrow = length(odeini), ncol = length(outtimes))
+    dimnames(o) <- list(names(odeini), NULL)
+    out <- cbind(time = outtimes, t(o))
+  } 
+  if (solution == "deSolve") {
+    out <- ode(
+      y = odeini,
+      times = outtimes,
+      func = fit$mkindiff, 
+      parms = odeparms,
+      atol = fit$atol
+    )
+  }
     
   # Output transformation for models with unobserved compartments like SFORB
   out_transformed <- data.frame(time = out[,"time"])
@@ -36,14 +85,16 @@ mkinplot <- function(fit, xlab = "Time", ylab = "Observed", xlim = range(fit$dat
   # Plot the data and model output
   plot(0, type="n", 
     xlim = xlim, ylim = ylim,
-      xlab = xlab, ylab = ylab, ...)
-    col_obs <- pch_obs <- 1:length(fit$map)
-    names(col_obs) <- names(pch_obs) <- names(fit$map)
-    for (obs_var in names(fit$map)) {
-      points(subset(fit$data, variable == obs_var, c(time, observed)), 
-        pch = pch_obs[obs_var], col = col_obs[obs_var])
-    }
-    matlines(out_transformed$time, out_transformed[-1])
-      legend("topright", inset=c(0.05, 0.05), legend=names(fit$map),
+    xlab = xlab, ylab = ylab, ...)
+  col_obs <- pch_obs <- 1:length(fit$map)
+  names(col_obs) <- names(pch_obs) <- names(fit$map)
+  for (obs_var in names(fit$map)) {
+    points(subset(fit$data, variable == obs_var, c(time, observed)), 
+    pch = pch_obs[obs_var], col = col_obs[obs_var])
+  }
+  matlines(out_transformed$time, out_transformed[-1])
+  if (legend == TRUE) {
+    legend("topright", inset=c(0.05, 0.05), legend=names(fit$map),
       col=col_obs, pch=pch_obs, lty=1:length(pch_obs))
+  }
 }
diff --git a/R/mkinresplot.R b/R/mkinresplot.R
new file mode 100644
index 0000000..bede5f7
--- /dev/null
+++ b/R/mkinresplot.R
@@ -0,0 +1,54 @@
+# $Id:  $
+
+# Copyright (C) 2008-2011 Katrin Lindenberger and Johannes Ranke
+# Contact: mkin-devel@lists.berlios.de
+
+# This file is part of the R package mkin
+
+# mkin is free software: you can redistribute it and/or modify it under the
+# terms of the GNU General Public License as published by the Free Software
+# Foundation, either version 3 of the License, or (at your option) any later
+# version.
+
+# This program is distributed in the hope that it will be useful, but WITHOUT
+# ANY WARRANTY; without even the implied warranty of MERCHANTABILITY or FITNESS
+# FOR A PARTICULAR PURPOSE.  See the GNU General Public License for more
+# details.
+
+# You should have received a copy of the GNU General Public License along with
+# this program. If not, see <http://www.gnu.org/licenses/>
+
+mkinresplot <- function (object, obs_vars = vector(), 
+  xlab = "Time [days]", ylab = "Residual [% of applied radioactivity]",
+	maxabs = "auto", legend= TRUE, lpos = "topright", ...) 
+{
+	obs_vars_all <- as.character(unique(object$data$variable))
+
+  if (length(obs_vars) > 0){
+      vars <- intersect(obs_vars_all, obs_vars)	
+  } else vars <- obs_vars_all
+
+  residuals <- subset(object$data, variable %in% vars, residual)
+
+  if (maxabs == "auto") maxabs = max(abs(residuals), na.rm = TRUE)
+
+	col_obs <- pch_obs <- 1:length(vars)
+ 	names(col_obs) <- names(pch_obs) <- vars
+
+  plot(0,  xlab = xlab, ylab = ylab, 
+       xlim = c(0, 1.1 * max(object$data$time)), 
+       ylim = c(-1.2 * maxabs, 1.2 * maxabs), ...)
+
+	for(var in vars){
+		residuals_plot <- subset(object$data, variable == var, c("time", "residual"))
+		points(residuals_plot, pch = pch_obs[var], col = col_obs[var])
+	}
+
+  abline(h = 0, lty = 2)
+  title(paste("Residuals of mkin fit"), font.main = 1)
+
+ 	if (legend == TRUE) {
+    legend(lpos, inset = c(0.05, 0.05), legend = vars, 
+    col = col_obs, pch = pch_obs)
+  }
+}
diff --git a/R/mkinstart.R b/R/mkinstart.R
new file mode 100644
index 0000000..46e5bed
--- /dev/null
+++ b/R/mkinstart.R
@@ -0,0 +1,23 @@
+mkinstart <- function(model, data, mode = "auto")
+{
+  if (class(model) != "mkinmod") stop("The first argument must be a model of class mkinmod")
+  names <- model$parms
+  observed <- names(model$map)
+  if(!all(observed %in% levels(data$name))) stop("The data must contain the observed variables used in the model")
+  for (obs in observed)
+  {
+    tmp <- subset(data, name == obs)
+    max <- tmp[which.max(tmp$value), ]
+    type = names(model$map[[obs]])[[1]]
+    kinmodel <- ifelse(type == "SFORB", "DFOP", type)
+    tmp.longdata <- subset(data, name == obs & time >= max$time)
+    tmp.widedata <- mkin_long_to_wide(tmp.longdata, outtime = "t")
+    names(tmp.widedata) <- c("t", "parent")
+    tmp.fit <- kinfit(
+      kindata = tmp.widedata,
+      kinmodels = kinmodel,
+      parent.0.user = max$value)
+    if(class(tmp.fit[[kinmodel]]) == "try-error") stop(paste("Automatic generation of starting parameters failed\nkinfit failed to find a", kinmodel, "fit for", obs))
+    tmp.results <- kinresults(tmp.fit)
+  }
+}
diff --git a/inst/GUI/.RData b/inst/GUI/.RData
new file mode 100644
index 0000000..2e82ef7
Binary files /dev/null and b/inst/GUI/.RData differ
diff --git a/inst/GUI/.Rhistory b/inst/GUI/.Rhistory
new file mode 100644
index 0000000..0704745
--- /dev/null
+++ b/inst/GUI/.Rhistory
@@ -0,0 +1,3 @@
+require(gWidgetsWWW)
+localServerStart("simple.R")
+quit("yes")
diff --git a/inst/GUI/gdf-test.R b/inst/GUI/gdf-test.R
new file mode 100644
index 0000000..b1ec20a
--- /dev/null
+++ b/inst/GUI/gdf-test.R
@@ -0,0 +1,12 @@
+w <- gwindow("gdf test")
+g <- ggroup(horizontal=FALSE, cont=w)
+d <- gdf(data.frame(a=c(1.1, 2.2, 3.3), b= c("one", "two", "three"), stringsAsFactors=FALSE), 
+  name = "Test for editing character columns", cont=g)
+size(d) <- c(400,400)
+gbutton("Change [1,2]", handler=function(h,...) {
+  d[1,2] <- "test"
+}, container=g)
+gbutton("Value of [1,2]", handler=function(h,...) {
+  galert(d[1,2], parent=d)
+}, cont=g)
+visible(w) <- TRUE
diff --git a/inst/GUI/simple-Gtk.R b/inst/GUI/simple-Gtk.R
new file mode 100644
index 0000000..8affdcc
--- /dev/null
+++ b/inst/GUI/simple-Gtk.R
@@ -0,0 +1,33 @@
+# Work in progress - simple Gtk2 GUI for mkin
+require(gWidgets)
+options("guiToolkit"="RGtk2")
+
+w <- gwindow("Simple R GUI for kinetic evaluations",
+  width=800, height=500)
+
+# Project definition expanding group
+pr <- gexpandgroup("Project definition", container=w)
+
+n.observed <- 1
+max.n.observed <- 9
+observed.names = c("parent", paste("M", 1:(max.n.observed - 1), sep=""))
+
+prg <- ggroup(horizontal=FALSE, cont = w)
+prl <- glayout(cont = prg)
+prl[1,1] <- glabel("Number of observed variables", cont=prl)
+prl[1,2] <- (n.observed.gw = gcombobox(
+  1:max.n.observed, 
+  handler = function(h, ...) {
+    n.observed <- svalue(n.observed.gw)
+    visible(observed.gw) <- c(
+      rep(TRUE, svalue(n.observed)), 
+      rep(FALSE, max.n.observed - n.observed))
+  },
+  cont=prl))
+
+observed.gw <- gdf(
+  items = data.frame(Index = 1:max.n.observed, 
+    Name = observed.names, stringsAsFactors=FALSE),
+  name = "Names of observed variables",
+  cont=prg)
+
diff --git a/inst/GUI/simple.R b/inst/GUI/simple.R
new file mode 100644
index 0000000..c187414
--- /dev/null
+++ b/inst/GUI/simple.R
@@ -0,0 +1,68 @@
+# Work in progress - simple GUI for mkin
+w <- gwindow('Simple R GUI for kinetic evaluations', visible=FALSE) 
+# Project definition {{{
+pr <- gexpandgroup("Project", cont=w)
+
+n.observed <- 1
+max.n.observed <- 9
+observed.names = c("parent", paste("M", 1:(max.n.observed - 1), sep=""))
+
+prg <- ggroup(horizontal=FALSE, cont = pr)
+prl <- glayout(cont = prg)
+prl[1,1] <- glabel("Number of observed variables", cont=prl)
+prl[1,2] <- (n.observed.gw = gcombobox(
+  1:max.n.observed, 
+  handler = function(h, ...) {
+    n.observed <<- svalue(n.observed.gw)
+    filter.expression <- paste("^[1-", n.observed, "]$", sep="")
+    observed.gw$filter("Index", filter.expression)
+  },
+  cont=prl))
+
+observed.gw <- gdf(
+  items = data.frame(Index = 1:max.n.observed, 
+    Name = observed.names, stringsAsFactors=FALSE),
+  name = "Names of observed variables",
+  width = 500, height=250, cont=prg)
+
+addSpace(prg, 15)
+prf <- gfile("Project file in binary R format (preferably use .RData as extension)", 
+  container = prg)
+addSpring(prg)
+addSpace(prg, 15)
+pr.ok <- gbutton("save", 
+  handler=function(h,...) {
+      galert(svalue(prf), parent=w)
+    }, container=prg)
+
+gbutton("ok", handler = function(h, ...) {
+  observed <- observed.gw[1:n.observed,2]
+  save(observed, file="observed.RData")
+  visible(pr) <- FALSE
+  },
+  cont=prg
+)
+
+visible(pr) <- TRUE
+# }}}
+
+# Dataset definition
+ds <- gexpandgroup("Datasets", cont=w)
+s <- gdf(data.frame( Author = c("Meier"), Year = "3", Title = "4"),
+  name = "Studies",
+cont=ds)
+
+size(s) <- c(800,200)
+visible(ds) <- TRUE
+
+# Model definition
+ms <- gexpandgroup("Models", cont=w)
+visible(ms) <- FALSE
+
+# Evaluation window
+mw <- gframe("Evaluations", cont=w)
+
+# Status bar
+gstatusbar("Powered by gWidgetsWWW", cont = w)
+visible(w) <- TRUE 
+# vim: set foldmethod=marker:
diff --git a/inst/GUI/test.R b/inst/GUI/test.R
new file mode 100644
index 0000000..e33e077
--- /dev/null
+++ b/inst/GUI/test.R
@@ -0,0 +1,17 @@
+require(gWidgetsWWW)
+localServerStart("simple.R")
+
+localServerStart("gdf-test.R")
+localServerStart("gdf-test-john.R")
+
+localServerStart("Examples/ex-actions.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-add-widget-dynamically.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-clt.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-form.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-gcombobox.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-gtable.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-index.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-layouts.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-simple-gui.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-widgets.R", package="gWidgetsWWW")
+localServerStart("Examples/ex-windows.R", package="gWidgetsWWW")
diff --git a/inst/doc/Rplots.pdf b/inst/doc/Rplots.pdf
new file mode 100644
index 0000000..a6ed15e
--- /dev/null
+++ b/inst/doc/Rplots.pdf
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diff --git a/inst/doc/mkin.Rnw b/inst/doc/mkin.Rnw
index 78b59e6..2f71151 100644
--- a/inst/doc/mkin.Rnw
+++ b/inst/doc/mkin.Rnw
@@ -1,3 +1,4 @@
+% $Id: mkin.Rnw 66 2010-09-03 08:50:26Z jranke $
 %%\VignetteIndexEntry{Routines for fitting kinetic models with one or more state variables to chemical degradation data}
 %%VignetteDepends{FME}
 %%\usepackage{Sweave}
@@ -78,7 +79,7 @@ barrier for \RR{} newcomers.
 \subsection{Data format}
 
 The following listing shows example dataset C from the FOCUS kinetics
-report as distributed with the \Rpackage{kinfit} package
+report as distributed with the \Rpackage{mkin} package
 
 <<FOCUS_2006_C_data, echo=TRUE, eval=TRUE>>=
 library("mkin")
@@ -101,8 +102,9 @@ as shown in the following listing
 
 <<data_format, echo=TRUE>>=
 example_data <- data.frame(
+  name = rep("parent", 9),
   time = c(0, 1, 3, 7, 14, 28, 63, 91, 119),
-  parent = c(85.1, 57.9, 29.9, 14.6, 9.7, 6.6, 4, 3.9, 0.6)
+  value = c(85.1, 57.9, 29.9, 14.6, 9.7, 6.6, 4, 3.9, 0.6)
 )
 @
 
@@ -122,12 +124,23 @@ SFORB_SFO <- mkinmod(
   m1 = list(type = "SFO"))
 @
 
+The model definitions given above define sets of linear first-order ordinary
+differential equations. In these cases, a coefficient matrix is also returned.
+
+Other models that include time on the right-hand side of the differential 
+equation are the first-order multi-compartment (FOMC) model and the
+Hockey-Stick (HS) model. At present, only the FOMC model can only be used, and
+only for the parent compound.
+
 \subsection{Fitting the model}
 
 Then the model parameters should be fitted to the data. The function
 \Robject{mkinfit} internally creates a cost function using \Robject{modCost}
 from the \Rpackage{FME} package and the produces a fit using \Robject{modFit}
-from the same package.
+from the same package. In cases of linear first-order differential 
+equations, the solution used for calculating the cost function is based
+on the fundamental system of the coefficient matrix, as proposed by 
+\citet{bates88}.
 
 <<model_fitting, echo=TRUE>>=
 # Do not show significance stars as they interfere with vignette generation
@@ -136,8 +149,10 @@ SFO.fit <- mkinfit(SFO, FOCUS_2006_C)
 summary(SFO.fit)
 SFORB.fit <- mkinfit(SFORB, FOCUS_2006_C)
 summary(SFORB.fit)
-SFO_SFO.fit <- mkinfit(SFO_SFO, FOCUS_2006_D)
-summary(SFO_SFO.fit)
+SFO_SFO.fit <- mkinfit(SFO_SFO, FOCUS_2006_D, plot=TRUE)
+summary(SFO_SFO.fit, data=FALSE)
+SFORB_SFO.fit <- mkinfit(SFORB_SFO, FOCUS_2006_D, plot=TRUE)
+summary(SFORB_SFO.fit, data=FALSE)
 @
 
 \bibliographystyle{plainnat}
diff --git a/inst/doc/mkin.pdf b/inst/doc/mkin.pdf
index 4d2e1d1..f963d1e 100644
Binary files a/inst/doc/mkin.pdf and b/inst/doc/mkin.pdf differ
diff --git a/inst/doc/references.bib b/inst/doc/references.bib
index b158eeb..24672e2 100644
--- a/inst/doc/references.bib
+++ b/inst/doc/references.bib
@@ -53,3 +53,10 @@
   address       = {Piacenza},
   pages         = {916--923}
 }
+
+@Book{            bates88,
+  title         = {Nonlinear regression and its applications},
+  author        = {D. Bates and D. Watts},
+  year          = {1988},
+  publisher     = {Wiley-Interscience}
+}
diff --git a/inst/unitTests/runit.mkinfit.R b/inst/unitTests/runit.mkinfit.R
index df09cc6..831c069 100644
--- a/inst/unitTests/runit.mkinfit.R
+++ b/inst/unitTests/runit.mkinfit.R
@@ -1,3 +1,23 @@
+# $Id: runit.mkinfit.R 68 2010-09-09 22:40:04Z jranke $
+
+# Copyright (C) 2010 Johannes Ranke
+# Contact: mkin-devel@lists.berlios.de
+
+# This file is part of the R package mkin
+
+# mkin is free software: you can redistribute it and/or modify it under the
+# terms of the GNU General Public License as published by the Free Software
+# Foundation, either version 3 of the License, or (at your option) any later
+# version.
+
+# This program is distributed in the hope that it will be useful, but WITHOUT
+# ANY WARRANTY; without even the implied warranty of MERCHANTABILITY or FITNESS
+# FOR A PARTICULAR PURPOSE.  See the GNU General Public License for more
+# details.
+
+# You should have received a copy of the GNU General Public License along with
+# this program. If not, see <http://www.gnu.org/licenses/>
+
 test.mkinmod.schaefer07_complex_example <- function()
 {
   schaefer07_complex_model <- mkinmod(
@@ -17,16 +37,16 @@ test.mkinmod.schaefer07_complex_example <- function()
   r$mkin <- c(
     k_parent,
     s$distimes["parent", "DT50"],
-    k_parent_A1/k_parent,
+    s$ff["parent_A1"],
     sum(k_A1_sink, k_A1_A2),
     s$distimes["A1", "DT50"],
-    k_parent_B1/k_parent,
+    s$ff["parent_B1"],
     k_B1_sink,
     s$distimes["B1", "DT50"],
-    k_parent_C1/k_parent,
+    s$ff["parent_C1"],
     k_C1_sink,
     s$distimes["C1", "DT50"],
-    k_A1_A2/(k_A1_A2 + k_A1_sink),
+    s$ff["A1_A2"],
     k_A2_sink,
     s$distimes["A2", "DT50"])
   r$means <- (r$KinGUI + r$ModelMaker)/2
diff --git a/inst/unitTests/runit.mkinmod.R b/inst/unitTests/runit.mkinmod.R
index 44d9ffb..a0e8996 100644
--- a/inst/unitTests/runit.mkinmod.R
+++ b/inst/unitTests/runit.mkinmod.R
@@ -1,3 +1,23 @@
+# $Id: runit.mkinmod.R 64 2010-09-01 13:33:51Z jranke $
+
+# Copyright (C) 2010 Johannes Ranke
+# Contact: mkin-devel@lists.berlios.de
+
+# This file is part of the R package mkin
+
+# mkin is free software: you can redistribute it and/or modify it under the
+# terms of the GNU General Public License as published by the Free Software
+# Foundation, either version 3 of the License, or (at your option) any later
+# version.
+
+# This program is distributed in the hope that it will be useful, but WITHOUT
+# ANY WARRANTY; without even the implied warranty of MERCHANTABILITY or FITNESS
+# FOR A PARTICULAR PURPOSE.  See the GNU General Public License for more
+# details.
+
+# You should have received a copy of the GNU General Public License along with
+# this program. If not, see <http://www.gnu.org/licenses/>
+
 test.mkinmod.SFO <- function()
 {  
   SFO.diffs <- c(
@@ -5,7 +25,9 @@ test.mkinmod.SFO <- function()
   )
   SFO.parms <- c("k_parent_sink")
   SFO.map <- list(parent = c(SFO = "parent"))
-  SFO <- list(diffs = SFO.diffs, parms = SFO.parms, map = SFO.map)
+  SFO.coefmat <- matrix("- k_parent_sink", dimnames = list("parent", "parent"))
+  SFO <- list(diffs = SFO.diffs, parms = SFO.parms, map = SFO.map, 
+    coefmat = SFO.coefmat)
   class(SFO) <- "mkinmod"
   SFO.1 <- mkinmod(
     parent = list(type = "SFO", to = NULL, sink = TRUE)
@@ -39,7 +61,13 @@ test.mkinmod.SFORB <- function()
   )
   SFORB.parms <- c("k_parent_free_sink", "k_parent_free_bound", "k_parent_bound_free")
   SFORB.map <- list(parent = c(SFORB = "parent_free", SFORB = "parent_bound"))
-  SFORB <- list(diffs = SFORB.diffs, parms = SFORB.parms, map = SFORB.map)
+  vars <- paste("parent", c("free", "bound"), sep="_")
+  SFORB.coefmat <- matrix(
+    c("- k_parent_free_sink - k_parent_free_bound", "k_parent_bound_free",
+      "k_parent_free_bound", "- k_parent_bound_free"), nrow=2, byrow=TRUE, 
+    dimnames=list(vars, vars))
+  SFORB <- list(diffs = SFORB.diffs, parms = SFORB.parms, 
+    map = SFORB.map, coefmat = SFORB.coefmat)
   class(SFORB) <- "mkinmod"
   SFORB.mkinmod <- mkinmod(
     parent = list(type = "SFORB", to = NULL, sink=TRUE)
@@ -55,7 +83,12 @@ test.mkinmod.SFO_SFO <- function()
   )
   SFO_SFO.parms <- c("k_parent_sink", "k_m1_sink", "k_parent_m1")
   SFO_SFO.map <- list(parent = c(SFO = "parent"), m1 = c(SFO = "m1"))
-  SFO_SFO <- list(diffs = SFO_SFO.diffs, parms = SFO_SFO.parms, map = SFO_SFO.map)
+  vars <- c("parent", "m1")
+  SFO_SFO.coefmat <- matrix(c("- k_parent_sink - k_parent_m1", 
+          "0", "k_parent_m1", "- k_m1_sink"), nrow=2, byrow=TRUE,
+      dimnames=list(vars, vars))
+  SFO_SFO <- list(diffs = SFO_SFO.diffs, parms = SFO_SFO.parms, 
+    map = SFO_SFO.map, coefmat = SFO_SFO.coefmat)
   class(SFO_SFO) <- "mkinmod"
   SFO_SFO.mkinmod <- mkinmod(
     parent = list(type = "SFO", to = "m1", sink=TRUE),
@@ -73,7 +106,14 @@ test.mkinmod.SFO_SFO2 <- function()
   )
   SFO_SFO2.parms <- c("k_parent_sink", "k_m1_sink", "k_m2_sink", "k_parent_m1", "k_parent_m2")
   SFO_SFO2.map <- list(parent = c(SFO = "parent"), m1 = c(SFO = "m1"), m2 = c(SFO = "m2"))
-  SFO_SFO2 <- list(diffs = SFO_SFO2.diffs, parms = SFO_SFO2.parms, map = SFO_SFO2.map)
+  vars <- c("parent", "m1", "m2")
+  SFO_SFO2.coefmat <- matrix(
+      c("- k_parent_sink - k_parent_m1 - k_parent_m2", "0", "0",
+          "k_parent_m1", "- k_m1_sink", "0",
+          "k_parent_m2", "0", "- k_m2_sink"), nrow=3, byrow=TRUE,
+      dimnames=list(vars, vars))
+  SFO_SFO2 <- list(diffs = SFO_SFO2.diffs, parms = SFO_SFO2.parms, 
+      map = SFO_SFO2.map, coefmat = SFO_SFO2.coefmat)
   class(SFO_SFO2) <- "mkinmod"
   SFO_SFO2.mkinmod <- mkinmod(
     parent = list(type = "SFO", to = c("m1", "m2"), sink=TRUE),
@@ -90,9 +130,16 @@ test.mkinmod.FOMC_SFO2 <- function()
     m1 = "d_m1 = - k_m1_sink * m1 + f_to_m1 * (alpha/beta) * ((time/beta) + 1)^-1 * parent",
     m2 = "d_m2 = - k_m2_sink * m2 + (1 - f_to_m1) * f_to_m2 * (alpha/beta) * ((time/beta) + 1)^-1 * parent"
   )
-  FOMC_SFO2.parms <- c("alpha", "beta", "k_m1_sink", "k_m2_sink", "f_to_m1", "f_to_m2")
-  FOMC_SFO2.map <- list(parent = c(FOMC = "parent"), m1 = c(SFO = "m1"), m2 = c(SFO = "m2"))
-  FOMC_SFO2 <- list(diffs = FOMC_SFO2.diffs, parms = FOMC_SFO2.parms, map = FOMC_SFO2.map)
+  FOMC_SFO2.parms <- c("alpha", "beta", "k_m1_sink", "k_m2_sink", 
+    "f_to_m1", "f_to_m2")
+  FOMC_SFO2.map <- list(parent = c(FOMC = "parent"), 
+    m1 = c(SFO = "m1"), 
+    m2 = c(SFO = "m2"))
+  FOMC_SFO2.ff <- c(
+    m1 = "f_to_m1", 
+    m2 = "(1 - f_to_m1) * f_to_m2")
+  FOMC_SFO2 <- list(diffs = FOMC_SFO2.diffs, parms = FOMC_SFO2.parms, 
+    map = FOMC_SFO2.map, ff = FOMC_SFO2.ff)
   class(FOMC_SFO2) <- "mkinmod"
   FOMC_SFO2.mkinmod <- mkinmod(
     parent = list(type = "FOMC", to = c("m1", "m2"), sink=TRUE),
diff --git a/man/DFOP.solution.Rd b/man/DFOP.solution.Rd
new file mode 100644
index 0000000..d30cf7f
--- /dev/null
+++ b/man/DFOP.solution.Rd
@@ -0,0 +1,36 @@
+\name{DFOP.solution}
+\Rdversion{1.1}
+\alias{DFOP.solution}
+\title{
+Dual First-Order in Parallel kinetics
+}
+\description{
+  Function describing decline from a defined starting value using the sum
+  of two exponential decline functions.
+}
+\usage{
+DFOP.solution(t, parent.0, k1, k2, g)
+}
+\arguments{
+  \item{t}{ Time. }
+  \item{parent.0}{ Starting value for the response variable at time zero. }
+  \item{k1}{ First kinetic constant. }
+  \item{k2}{ Second kinetic constant. }
+  \item{g}{ Fraction of the starting value declining according to the
+    first kinetic constant.
+  }
+}
+\value{
+  The value of the response variable at time \code{t}.
+}
+\references{ 
+  FOCUS (2006) \dQuote{Guidance Document on Estimating Persistence and
+  Degradation Kinetics from Environmental Fate Studies on Pesticides in EU
+  Registration} Report of the FOCUS Work Group on Degradation Kinetics,
+  EC Document Reference Sanco/10058/2005 version 2.0, 434 pp,
+  \url{http://focus.jrc.ec.europa.eu/dk} 
+}
+\examples{
+  \dontrun{plot(function(x) DFOP.solution(x, 100, 5, 0.5, 0.3), 0, 4, ylim=c(0,100))}
+}
+\keyword{ manip }
diff --git a/man/FOCUS_2006_datasets.Rd b/man/FOCUS_2006_datasets.Rd
index 04565f7..5053b88 100644
--- a/man/FOCUS_2006_datasets.Rd
+++ b/man/FOCUS_2006_datasets.Rd
@@ -11,7 +11,7 @@
 Datasets A to F from the FOCUS Kinetics report from 2006
 }
 \description{
-Data taken from an FOCUS (2006), p. 258.
+Data taken from FOCUS (2006), p. 258.
 }
 \usage{FOCUS_2006_datasets}
 \format{
diff --git a/man/FOMC.solution.Rd b/man/FOMC.solution.Rd
new file mode 100644
index 0000000..d04d34e
--- /dev/null
+++ b/man/FOMC.solution.Rd
@@ -0,0 +1,49 @@
+\name{FOMC.solution}
+\Rdversion{1.1}
+\alias{FOMC.solution}
+\title{ First-Order Multi-Compartment kinetics }
+\description{
+  Function describing exponential decline from a defined starting value, with 
+  a decreasing rate constant. 
+
+  The form given here differs slightly from the original reference by Gustafson
+  and Holden (1990). The parameter \code{beta} corresponds to 1/beta in the
+  original equation.
+}
+\usage{
+FOMC.solution(t, parent.0, alpha, beta)
+}
+\arguments{
+  \item{t}{ Time. }
+  \item{parent.0}{ Starting value for the response variable at time zero. }
+  \item{alpha}{ 
+    Shape parameter determined by coefficient of variation of rate constant
+    values. }
+  \item{beta}{
+    Location parameter.
+}
+}
+\note{
+  The solution of the FOMC kinetic model reduces to the
+  \code{\link{SFO.solution}} for large values of \code{alpha} and
+  \code{beta} with 
+  \eqn{k = \frac{\beta}{\alpha}}{k = beta/alpha}.
+}
+\value{
+  The value of the response variable at time \code{t}.
+}
+\references{
+  FOCUS (2006) \dQuote{Guidance Document on Estimating Persistence and
+  Degradation Kinetics from Environmental Fate Studies on Pesticides in EU
+  Registration} Report of the FOCUS Work Group on Degradation Kinetics,
+  EC Document Reference Sanco/10058/2005 version 2.0, 434 pp,
+  \url{http://focus.jrc.ec.europa.eu/dk} 
+
+  Gustafson DI and Holden LR (1990) Nonlinear pesticide dissipation in soil: A
+  new model based on spatial variability. \emph{Environmental Science and 
+  Technology} \bold{24}, 1032-1038
+}
+\examples{
+  \dontrun{plot(function(x) FOMC.solution(x, 100, 10, 2), 0, 2)}
+}
+\keyword{ manip }
diff --git a/man/HS.solution.Rd b/man/HS.solution.Rd
new file mode 100644
index 0000000..71f68a1
--- /dev/null
+++ b/man/HS.solution.Rd
@@ -0,0 +1,34 @@
+\name{HS.solution}
+\Rdversion{1.1}
+\alias{HS.solution}
+\title{ Hockey-Stick kinetics }
+\description{
+  Function describing two exponential decline functions with a break point
+  between them.
+}
+\usage{
+HS.solution(t, parent.0, k1, k2, tb)
+}
+\arguments{
+  \item{t}{ Time. }
+  \item{parent.0}{ Starting value for the response variable at time zero. }
+  \item{k1}{ First kinetic constant. }
+  \item{k2}{ Second kinetic constant. }
+  \item{tb}{ Break point. Before this time, exponential decline according
+    to \code{k1} is calculated, after this time, exponential decline proceeds
+    according to \code{k2}. }
+}
+\value{
+  The value of the response variable at time \code{t}.
+}
+\references{ 
+  FOCUS (2006) \dQuote{Guidance Document on Estimating Persistence and
+  Degradation Kinetics from Environmental Fate Studies on Pesticides in EU
+  Registration} Report of the FOCUS Work Group on Degradation Kinetics,
+  EC Document Reference Sanco/10058/2005 version 2.0, 434 pp,
+  \url{http://focus.jrc.ec.europa.eu/dk} 
+}
+\examples{
+  \dontrun{plot(function(x) HS.solution(x, 100, 2, 0.3, 0.5), 0, 2, ylim=c(0,100))}
+}
+\keyword{ manip }
diff --git a/man/SFO.solution.Rd b/man/SFO.solution.Rd
new file mode 100644
index 0000000..41a9ba9
--- /dev/null
+++ b/man/SFO.solution.Rd
@@ -0,0 +1,29 @@
+\name{SFO.solution}
+\Rdversion{1.1}
+\alias{SFO.solution}
+\title{ Single First-Order kinetics }
+\description{
+  Function describing exponential decline from a defined starting value.
+}
+\usage{
+  SFO.solution(t, parent.0, k)
+}
+\arguments{
+  \item{t}{ Time. }
+  \item{parent.0}{ Starting value for the response variable at time zero. }
+  \item{k}{ Kinetic constant. }
+}
+\value{
+  The value of the response variable at time \code{t}.
+}
+\references{ 
+  FOCUS (2006) \dQuote{Guidance Document on Estimating Persistence and
+  Degradation Kinetics from Environmental Fate Studies on Pesticides in EU
+  Registration} Report of the FOCUS Work Group on Degradation Kinetics,
+  EC Document Reference Sanco/10058/2005 version 2.0, 434 pp,
+  \url{http://focus.jrc.ec.europa.eu/dk} 
+}
+\examples{
+  \dontrun{plot(function(x) SFO.solution(x, 100, 3), 0, 2)}
+}
+\keyword{ manip }
diff --git a/man/SFORB.solution.Rd b/man/SFORB.solution.Rd
new file mode 100644
index 0000000..a935f69
--- /dev/null
+++ b/man/SFORB.solution.Rd
@@ -0,0 +1,36 @@
+\name{SFORB.solution}
+\Rdversion{1.1}
+\alias{SFORB.solution}
+\title{ Single First-Order Reversible Binding kinetics }
+\description{
+  Function describing the solution of the differential equations describing
+  the kinetic model with first-order terms for a two-way transfer from a free
+  to a bound fraction, and a first-order degradation term for the free
+  fraction.  The initial condition is a defined amount in the free fraction and
+  no substance in the bound fraction.
+}
+\usage{
+  SFORB.solution(t, parent.0, k_12, k_21, k_1output)
+}
+\arguments{
+  \item{t}{ Time. }
+  \item{parent.0}{ Starting value for the response variable at time zero. }
+  \item{k_12}{ Kinetic constant describing transfer from free to bound. }
+  \item{k_21}{ Kinetic constant describing transfer from bound to free. }
+  \item{k_1output}{ Kinetic constant describing degradation of the free fraction. }
+}
+\value{
+  The value of the response variable, which is the sum of free and bound 
+  fractions at time \code{t}.
+}
+\references{ 
+  FOCUS (2006) \dQuote{Guidance Document on Estimating Persistence and
+  Degradation Kinetics from Environmental Fate Studies on Pesticides in EU
+  Registration} Report of the FOCUS Work Group on Degradation Kinetics,
+  EC Document Reference Sanco/10058/2005 version 2.0, 434 pp,
+  \url{http://focus.jrc.ec.europa.eu/dk} 
+}
+\examples{
+  \dontrun{plot(function(x) SFORB.solution(x, 100, 0.5, 2, 3), 0, 2)}
+}
+\keyword{ manip }
diff --git a/man/mkin_long_to_wide.Rd b/man/mkin_long_to_wide.Rd
index 97791e6..6fa1860 100644
--- a/man/mkin_long_to_wide.Rd
+++ b/man/mkin_long_to_wide.Rd
@@ -4,7 +4,7 @@
   Convert a dataframe from long to wide format.
 }
 \usage{
-mkin_long_to_wide(long_data, time = "time")
+mkin_long_to_wide(long_data, time = "time", outtime = "time")
 }
 \description{
   This function takes a dataframe in the long form as required by \code{\link{modCost}} 
@@ -17,7 +17,10 @@ mkin_long_to_wide(long_data, time = "time")
   \code{time} argument and one column of observed values named "value".
 }
   \item{time}{
-  The name of the time variable.
+  The name of the time variable in the long input data.
+}
+  \item{outtime}{
+  The name of the time variable in the wide output data.
 }
 }
 \value{
diff --git a/man/mkinerrmin.Rd b/man/mkinerrmin.Rd
index 4bbf96a..654115b 100644
--- a/man/mkinerrmin.Rd
+++ b/man/mkinerrmin.Rd
@@ -42,5 +42,4 @@ mkinerrmin(errdata, n.parms, alpha = 0.05)
   EC Document Reference Sanco/10058/2005 version 2.0, 434 pp,
   \url{http://focus.jrc.ec.europa.eu/dk} 
 }
-\author{ Johannes Ranke }
 \keyword{ manip }
diff --git a/man/mkinfit.Rd b/man/mkinfit.Rd
index 0ec2d21..d4139eb 100644
--- a/man/mkinfit.Rd
+++ b/man/mkinfit.Rd
@@ -15,7 +15,10 @@ mkinfit(mkinmod, observed,
   state.ini = c(100, rep(0, length(mkinmod$diffs) - 1)), 
   lower = 0, upper = Inf, 
   fixed_parms = NULL, fixed_initials = names(mkinmod$diffs)[-1], 
-  plot = FALSE, quiet = FALSE, err = NULL, weight = "none", scaleVar = FALSE, ...)
+  eigen = FALSE,
+  plot = FALSE, quiet = FALSE, err = NULL, weight = "none", 
+  scaleVar = FALSE, 
+  atol = 1e-6, ...)
 }
 \arguments{
   \item{mkinmod}{
@@ -32,8 +35,11 @@ mkinfit(mkinmod, observed,
     \code{\link{modFit}}.
   }
   \item{parms.ini}{
-    A named vector if initial values for the parameters, including both parameters to
+    A named vector if initial values for the parameters, including parameters to
     be optimised and potentially also fixed parameters as indicated by \code{fixed_parms}.
+    The default is to set the initial values to 0.1. The setting of the initial values for 
+    the parameters has a strong impart on performance and it lies in the responsibilty of the 
+    user to set sensible initial values.   
   }
   \item{state.ini}{
     A named vector of initial values for the state variables of the model. In case the 
@@ -47,9 +53,10 @@ mkinfit(mkinmod, observed,
     negative values to not make sense for the models currently created by \code{\link{mkinmod}}.
   }
   \item{upper}{
-    Upper bounds for the parameters, passed to \code{\link{modFit}}. Defaults to \code{Inf}. Setting
-    non-infinite upper bounds has a strong impact on performance, and using a method like "L-BFGS-B" (by 
-    specifying an additional \code{method} argument) is recommended.
+    Upper bounds for the parameters, passed to \code{\link{modFit}}. Defaults to \code{Inf} 
+    except for formation fraction parameters. Setting non-infinite upper bounds has a strong 
+    impact on performance, and using a method like "L-BFGS-B" (by specifying an additional 
+    \code{method} argument) is recommended.
   }
   \item{fixed_parms}{
     The names of parameters that should not be optimised but rather kept at the values
@@ -59,6 +66,12 @@ mkinfit(mkinmod, observed,
     The names of model variables for which the initial state at time 0 should be excluded
     from the optimisation. Defaults to all state variables except for the first one.
   }
+  \item{eigen}{
+    Should the solution of the system of differential equations be based on the 
+    spectral decomposition of the coefficient matrix in cases that this is
+    possible? Be aware that the results may differ from the results returned using
+    the ode solver.
+  }
   \item{plot}{
     Should the observed values and the numerical solutions be plotted at each stage
     of the optimisation?
@@ -77,13 +90,17 @@ mkinfit(mkinmod, observed,
     Will be passed to \code{\link{modCost}}. Default is not to scale Variables according
     to the number of observations.
   }
+  \item{atol}{
+    Absolute error tolerance, passed to \code{\link{ode}}. Default is 1e-6 as in 
+    \code{\link{lsoda}}.
+  }
   \item{\dots}{
     Further arguments that will be passed to \code{\link{modFit}}. 
   }
 }
 \value{
-    A list with "mkinfit" and "modFit" in the class attribute. Thus, at
-    present, a summary can be obtained by \code{\link{summary.modFit}}. 
+    A list with "mkinfit" and "modFit" in the class attribute. 
+    A summary can be obtained by \code{\link{summary.mkinfit}}. 
 }
 \author{
   Johannes Ranke <jranke@{harlan.com,uni-bremen.de}>
diff --git a/man/mkinmod.Rd b/man/mkinmod.Rd
index 7ec9627..7c11735 100644
--- a/man/mkinmod.Rd
+++ b/man/mkinmod.Rd
@@ -15,13 +15,16 @@ mkinmod(...)
   \item{...}{
     For each observed variable, a list has to be specified as an argument, containing
     at least a component \code{type}, specifying the type of kinetics to use
-    for the variable. Currently, only single first order kinetics "SFO" or
-    single first order with reversible binding "SFORB" are implemented, as well as
-    "FOMC" for the first compartment which is assumed to be the source compartment.
-    Optional components of each argument are \code{to}, a vector of names of
-    variables to which a transfer is to be assumed in the model, and
-    \code{sink}, a logical specifying if transformation to unspecified
-    compounds (sink) is to be assumed in the model (defaults to \code{TRUE})
+    for the variable. Currently, single first order kinetics "SFO" or
+    single first order with reversible binding "SFORB" are implemented for all
+    variables, while 
+    "FOMC", "DFOP" and "HS" can additionally be chosen for the first
+    variable which is assumed to be the source compartment.  Optional components
+    of each argument are \code{to}, a
+    vector of names of variables to which a transfer is to be assumed in the
+    model, and \code{sink}, a logical specifying if transformation to
+    unspecified compounds (sink) is to be assumed in the model (defaults to
+    \code{TRUE})
   }
 }
 \value{
@@ -31,6 +34,7 @@ mkinmod(...)
     \item{parms}{ A vector of parameter names occurring in the differential equations. }
     \item{map}{ A list containing named character vectors for each observed variable, specifying
       the modelling variables by which it is represented. }
+    \item{coefmat}{ The coefficient matrix, if the system of differential equations can be represented by one. }
 }
 \author{
   Johannes Ranke <jranke@{harlan.com,uni-bremen.de}>
diff --git a/man/mkinplot.Rd b/man/mkinplot.Rd
index 58959d7..b72675a 100644
--- a/man/mkinplot.Rd
+++ b/man/mkinplot.Rd
@@ -10,7 +10,8 @@
 }
 \usage{
   mkinplot(fit, xlab = "Time", ylab = "Observed", 
-    xlim = range(fit$data$time), ylim = range(fit$data$observed, na.rm=TRUE), ...)
+    xlim = range(fit$data$time), ylim = range(fit$data$observed, na.rm=TRUE), 
+    legend = TRUE, ...)
 }
 \arguments{
   \item{fit}{
@@ -28,6 +29,9 @@
   \item{ylim}{
     plot range in y direction.
   }
+  \item{legend}{
+    legend specifying if a legend should be included in the plot.
+  }
   \item{\dots}{
    further arguments passed to \code{\link{plot}}.
 }
diff --git a/man/mkinresplot.Rd b/man/mkinresplot.Rd
new file mode 100644
index 0000000..0b48692
--- /dev/null
+++ b/man/mkinresplot.Rd
@@ -0,0 +1,64 @@
+\name{mkinresplot}
+\alias{mkinresplot}
+\title{
+  Function to plot residuals stored in an mkin object
+}
+\description{
+  This function plots the residuals for the specified subset of the 
+  observed variables from an mkinfit object.
+}
+\usage{
+  mkinresplot(object, obs_vars = vector(), 
+    xlab = "Time [days]", ylab = "Residual [\% of applied radioactivity]", 
+    maxabs = "auto", legend = TRUE, lpos = "topright", ...)
+}
+\arguments{
+  \item{object}{
+    A fit represented in an \code{\link{mkinfit}} object.
+}
+  \item{obs_vars}{
+    A character vector of names of the observed variables for which residuals
+    should be plotted.
+}
+  \item{xlab}{
+    Label for the x axis. Defaults to "Time [days]".
+}
+  \item{ylab}{
+    Label for the y axis. Defaults to "Residual [\% of applied radioactivity]".
+}
+  \item{maxabs}{
+    Maximum absolute value of the residuals. This is used for the scaling of
+    the y axis and defaults to "auto".
+}
+  \item{legend}{
+    Should a legend be plotted? Defaults to "TRUE".
+}
+  \item{lpos}{ 
+    Where should the legend be placed? Default is "topright". Will be passed on to
+		\code{\link{legend}}. }
+  \item{\dots}{
+   further arguments passed to \code{\link{plot}}.
+}
+}
+\value{
+  Nothing is returned by this function, as it is called for its side effect, namely to produce a plot.
+}
+\author{
+  Katrin Lindenberger and Johannes Ranke
+}
+
+\seealso{
+ \code{\link{mkinplot}}, for a way to plot the data and the fitted lines of the
+ mkinfit object.  }
+\examples{
+data <- mkin_wide_to_long(schaefer07_complex_case, time = "time")
+model <- mkinmod(
+  parent = list(type = "SFO", to = c("A1", "B1", "C1"), sink = FALSE),
+  A1 = list(type = "SFO", to = "A2"),
+  B1 = list(type = "SFO"),
+  C1 = list(type = "SFO"),
+  A2 = list(type = "SFO"))
+\dontrun{fit <- mkinfit(model, data, plot=TRUE)}
+\dontrun{mkinresplot(fit, "A1")}
+}
+\keyword{ hplot }
diff --git a/man/mkinstart.Rd b/man/mkinstart.Rd
new file mode 100644
index 0000000..ec1204f
--- /dev/null
+++ b/man/mkinstart.Rd
@@ -0,0 +1,38 @@
+\name{mkinstart}
+\alias{mkinstart}
+\title{
+  Generate starting parameters for optimisations
+}
+\description{
+  This function is supposed to analyse a kinetic model and kinetic data in
+  order to generate suitable starting parameters for fitting the model.
+  It does not do anything really useful at the moment.
+}
+\usage{
+mkinstart(model, data, mode = "auto")
+}
+\arguments{
+  \item{model}{
+    A kinetic model of class \code{\link{mkinmod}}.
+}
+  \item{data}{
+    Kinetic data in wide format suitable for fitting with \code{\link{mkinfit}}.
+}
+  \item{mode}{
+    How the starting parameters should be generated. At the moment, only 
+    "auto" is supported, which internally uses \code{\link{kinfit}}. 
+}
+}
+\details{
+%%  ~~ If necessary, more details than the description above ~~
+}
+\value{
+  A named vector of starting parameters.
+}
+\author{
+  Johannes Ranke
+}
+\examples{
+   
+}
+\keyword{ manip }
diff --git a/man/summary.mkinfit.Rd b/man/summary.mkinfit.Rd
index 1c30589..8a8c6ab 100644
--- a/man/summary.mkinfit.Rd
+++ b/man/summary.mkinfit.Rd
@@ -11,8 +11,8 @@
   and residual values.
 }
 \usage{
-\method{summary}{mkinfit}(object, data = TRUE, distimes = TRUE, cov = FALSE, ...)
-\method{print}{summary.mkinfit}(x, digits = max(3, getOption("digits") - 3), ...)
+\method{summary}{mkinfit}(object, data = TRUE, distimes = TRUE, ff = TRUE, cov = FALSE, ...)
+\method{print}{summary.mkinfit}(x, digits = max(3, getOption("digits") - 3), tval = TRUE, ...)
 }
 
 \arguments{
@@ -26,13 +26,20 @@
   logical, indicating whether the data should be included in the summary. 
 }
   \item{distimes}{
-  logical, indicating whether DT50 and DT90 values shoule be included.
+  logical, indicating whether DT50 and DT90 values should be included.
+}
+  \item{ff}{
+  logical, indicating whether formation fractions should be included.
 }
   \item{cov}{
   logical, indicating whether parameter covariances should be calculated.
 Passed to \code{\link{summary.modFit}}.  }
   \item{digits}{
   Number of digits to use for printing
+}
+  \item{tval}{
+  Should the test statistic of the t-test for parameter significance be
+  printed? Defaults to \code{TRUE}. Saves vertical space if set to \code{FALSE}.
 }
   \item{\dots}{
   optional arguments passed to methods like \code{print}.
@@ -47,6 +54,7 @@ Passed to \code{\link{summary.modFit}}.  }
   \item{fixed }{The values of fixed parameters.}
   \item{errmin }{The chi2 error levels for each observed variable.}
   \item{disstimes }{The DT50 and DT90 values for each observed variable.}
+  \item{ff }{The estimated formation fractions derived from the fitted model.}
   The print method is called for its side effect, i.e. printing the summary.
 }
 \references{
@@ -57,7 +65,7 @@ Passed to \code{\link{summary.modFit}}.  }
   \url{http://focus.jrc.ec.europa.eu/dk} 
 }
 \author{
-  Johannes Ranke <jranke@harlan.com>
+  Johannes Ranke <jranke@{harlan.com,uni-bremen.de}>
 }
 \examples{
   summary(mkinfit(mkinmod(parent = list(type = "SFO")), FOCUS_2006_A))
diff --git a/tests/doRUnit.R b/tests/doRUnit.R
index e2ad4cd..ed3ef1d 100644
--- a/tests/doRUnit.R
+++ b/tests/doRUnit.R
@@ -1,17 +1,10 @@
+# $Id: doRUnit.R 96 2011-04-29 11:10:40Z jranke $
+# Adapted from a version around 2.9 of the rcdk package by Rajarshi Guha
 if(require("RUnit", quietly=TRUE)) {
  
-  ## --- Setup ---
- 
-  pkg <- "mkin" # <-- Change to package name!
-  if(Sys.getenv("RCMDCHECK") == "FALSE") {
-    ## Path to unit tests for standalone running under Makefile (not R CMD check)
-    ## PKG/tests/../inst/unitTests
-    path <- file.path(getwd(), "..", "inst", "unitTests")
-  } else {
-    ## Path to unit tests for R CMD check
-    ## PKG.Rcheck/tests/../PKG/unitTests
-    path <- system.file(package=pkg, "unitTests")
-  }
+  pkg <- "mkin"
+  path <- system.file(package=pkg, "unitTests")
+
   cat("\nRunning unit tests\n")
   print(list(pkg=pkg, getwd=getwd(), pathToUnitTests=path))
  
-- 
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